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Like the series that inspired it, Grey's Anatomy Soundtrack Vol. 3 ebbs and flows with songs that are sweet, quirky and heart-stirring. At its centerpiece is new and exclusive music from acclaimed singer-songwriter Mat Kearney, Grammy winner John Legend and the inimitable Gomez. The album's tracks, many of which can be heard during key emotional scenes over the course of the series, were chosen by the show's creator and executive producer, Shonda Rhimes, and executive producer Betsy Beers from a large pool of artists introduced to them by music supervisor Alex Patsavas. Among the record's many highlights are Legend's spare and compelling "Sun Comes Up," Gomez's moving "Moon And Sun," and poignant compositions from Grace Potter & The Nocturnals ("Falling Or Flying"), Paolo Nutini ("Million Faces") and Brandi Carlile ("The Story").